8,880 results match your criteria catalyst conversion


Multifunctional MnO/AgSbS Nanotheranostic Agent for Single-Laser-Triggered Tumor Synergistic Therapy in the NIR-II Biowindow.

ACS Appl Mater Interfaces 2022 Jan 20. Epub 2022 Jan 20.

General Surgery Department, The Radiology Department of Third Hospital of Shanxi Medical University, Shanxi Bethune Hospital, Shanxi Academy of Medical Sciences, Taiyuan 030032, China.

Regulating the level of reactive oxygen species (ROS) in a tumor is an efficient and innovative anticancer strategy. However, the therapeutic efficacy of ROS-based therapies, such as chemodynamic therapy (CDT) and photodynamic therapy (PDT), offers finite outcomes due to the oxygen dependence and limited concentration of hydrogen peroxide (HO) and overexpression of glutathione (GSH) within the tumor microenvironment (TME), so a single therapeutic strategy is insufficient to completely eliminate tumors. Therefore, we demonstrated an omnipotent nanoplatform MnO/AgSbS (abbreviated as MA) with strong optical absorbance in the NIR-II biowindow and oxygen self-sufficient ROS-mediated ability, which not only relieves tumor hypoxia significantly but also enhances the photothermal therapy (PTT)/PDT/CDT efficacy. Read More

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January 2022

Guanidyl-implanted UiO-66 as an efficient catalyst for the enhanced conversion of carbon dioxide into cyclic carbonates.

Dalton Trans 2022 Jan 20. Epub 2022 Jan 20.

The Key Laboratory of Functional Molecular Solids, Ministry of Education, Anhui Laboratory of Molecule-Based Materials (State Key Laboratory Cultivation Base), College of Chemistry and Materials Science, Anhui Normal University, Wuhu, Anhui 241002, P.R. China.

The development of heterogeneous catalysts for promoting epoxide cycloaddition with carbon dioxide is highly desirable for recycling CO and achieving the goal of carbon neutrality. Herein, we designed and synthesized Zr-based metal organic frameworks (MOFs) by implanting functional guanidyl into the framework mixing different molar ratios of 4-guanidinobenzoic acid (Gua) with 1,4-benzenedicarboxylic acid (BDC). Consequently, a small sized Zr-MOF (∼350 nm) can be prepared by implanting Gua with 20% molar ligands, denoted as UiO-66-Gua(). Read More

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January 2022

Quasihexagonal Platinum Nanodendrites Decorated over CoS -N-Doped Reduced Graphene Oxide for Electro-Oxidation of C1-, C2-, and C3-Type Alcohols.

Adv Sci (Weinh) 2022 Jan 20:e2105344. Epub 2022 Jan 20.

Graduate School, Department of Energy Storage/Conversion Engineering (BK21 FOUR), Hydrogen and Fuel Cell Research Center, Jeonbuk National University, Jeonju, Jeollabuk-do, 54896, Republic of Korea.

The development of efficient and highly durable materials for renewable energy conversion devices is crucial to the future of clean energy demand. Herein, cage-like quasihexagonal structured platinum nanodendrites decorated over the transition metal chalcogenide core (CoS )-N-doped graphene oxide ([email protected] -NrGO) through optimized shape engineering and structural control technology are fabricated. The prepared electrocatalyst of [email protected] -NrGO is effectively used as anodic catalyst for alcohol oxidation in direct liquid alcohol fuel cells. Read More

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January 2022

Robust MOF-derived carbon-supported bimetallic Ni-Co catalysts for aqueous phase hydrodeoxygenation of vanillin.

Dalton Trans 2022 Jan 20. Epub 2022 Jan 20.

State Key Laboratory of Chemical Resources Engineering, Beijing University of Chemical Technology, Beijing, 100029, China.

Currently, rapidly increasing consumption of fossil resources has propelled the upgrading of biomass as an alternative and sustainable technology to produce important chemicals and bio-oils. In this regard, the rational design of low-cost and robust supported metal-based catalysts that exhibit excellent catalytic hydrodeoxygenation (HDO) performance for the conversion of biomass is quite necessary. Herein, we developed hierarchical flower-like nitrogen-doped carbon layer-coated bimetallic Ni-Co nanoparticles, which were distributed over the carbonaceous matrix ([email protected]@C), a metal-organic framework (MOF) ZIF-67 precursor approach, assisted by the etching of Ni ions, hydrothermal treatment together with glucose, and following carbonization processes. Read More

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January 2022

Tris(imidazolyl) dicopper(I) complex and its reactivity to exert the catalytic oxidation of sterically hindered phenol substrates a [CuO] core.

Dalton Trans 2022 Jan 20. Epub 2022 Jan 20.

Department of Chemistry, National Sun Yat-sen University, Kaohsiung 80424, Taiwan.

The Cu ion ligated with histidine residues is a common active site motif of various Cu-containing metalloenzymes exerting versatile catalytic oxidation reactions. Due to the scarcity of structurally characterized biomimetic binuclear Cu(I)-imidazolyl complexes, the bonding interactions between the Cu(I) center and imidazolyl donor ligands as well as their stoichiometric/catalytic oxidation reactivities remain relatively unexplored. In this study, we successfully synthesized a tris(imidazolyl) dicopper(I) complex [Cu(μ-bimeta)Cu][PF] (1) characterized by single-crystal X-ray diffraction, cyclic voltammetry, and UV-vis absorption spectroscopy. Read More

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January 2022

Synthesis of methyl glycolate by hydrogenation of dimethyl oxalate with a P modified Co/SiO catalyst.

Chem Commun (Camb) 2022 Jan 19. Epub 2022 Jan 19.

Hangzhou Institute of Advanced studies, Zhejiang Normal University, 1108 Gengwen Road, Hangzhou 311231, China.

A P-modified Co/SiO catalyst was reported for the first time in the selective hydrogenation of dimethyl oxalate (DMO) to methyl glycolate (MG) reaction and the synthesized CoP/SiO exhibited 94.6% conversion of DMO and 88.1% selectivity to MG during a 300 h continuous test. Read More

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January 2022

A High Conductivity One-Dimensional π-d Conjugated Metal-Organic Framework with Efficient Polysulfide Trapping-Diffusion-Catalysis in Lithium-Sulfur Batteries.

Adv Mater 2022 Jan 18:e2108835. Epub 2022 Jan 18.

Catalonia Institute for Energy Research - IREC, Sant Adrià de Besòs, Barcelona, 08930, Spain.

The shuttling behaviour and sluggish conversion kinetics of the intermediate lithium polysulfides (LiPS) represent the main obstructions to the practical application of lithium-sulfur batteries (LSBs). Herein, we present a one-dimensional (1D) π-d conjugated metal-organic framework, Ni-MOF-1D, as an efficient sulfur host to overcome these limitations. Experimental results and density functional theory (DFT) calculations demonstrate that Ni-MOF-1D is characterized by a remarkable binding strength for trapping soluble LiPS species. Read More

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January 2022

A Keggin-type polyoxometalate-based metal-organic complex as a highly efficient heterogeneous catalyst for the selective oxidation of alkylbenzenes.

Dalton Trans 2022 Jan 19. Epub 2022 Jan 19.

College of Chemistry and Materials Engineering, Bohai University, Jinzhou, 121013, P. R. China.

The direct oxidation of C-H bonds in organic materials into necessary oxygen-containing compounds under mild conditions has attracted increasing attention. A Keggin-type polyoxometalate-based metal-organic complex (MOC), [CuII4Cu(Htrz)(CO)(HO)(HPWCuII0.82O)]·8HO (1) (Htrz = 1,2,4-triazole), was designed and synthesized under hydrothermal conditions, and was structurally characterized by single crystal X-ray diffraction, PXRD, IR spectroscopy, TGA, and XPS. Read More

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January 2022

Coupling fine Pt nanoparticles and Co-N moiety as a synergistic bi-active site catalyst for oxygen reduction reaction in acid media.

J Colloid Interface Sci 2022 Jan 10;613:276-284. Epub 2022 Jan 10.

MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage, School of Chemistry and Chemical Engineering, State Key Lab of Urban Water Resource and Environment, Harbin Institute of Technology, Harbin, Heilongjiang 150001, China; Shenzhen Key Laboratory of Special Functional Materials, Shenzhen Engineering Laboratory for Advance Technology of Ceramics, Guangdong Research Center for Interfacial Engineering of Functional Materials, College of Materials Science and Engineering, Shenzhen University, Shenzhen 518060, China. Electronic address:

Fabricating high-efficiency catalysts of Pt nanoparticles coupled with single-atom sites (MNC) attracts intensive attention to accelerate the oxygen reduction reaction (ORR). Here we rationally design the low-Pt hybrid catalyst containing fine Pt nanoparticles coupled with Co-N moieties via a microwave-assisted heating process. The well-dispersed Pt nanoparticles are anchored by CoNC supports because of the metal-support interaction. Read More

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January 2022

Random Occupation of Multi-Metal Sites in Transition Metal-Organic Frameworks for Boosting Water Oxidation.

Chemistry 2022 Jan 18. Epub 2022 Jan 18.

Technical University of Denmark: Danmarks Tekniske Universitet, Department of Environmental Engineering, Bygningstorvet, Building 115, 2800, Kgs. Lyngby, DENMARK.

Developing robust oxygen evolution reaction (OER) electrocatalysts with excellent performance is essential for conversion of renewable electricity to clean fuel. Herein, we present a facile concept for the design of efficient high entropy metal-organic frameworks (HEMOFs) as electrocatalyst by one-step solvothermal synthesis. The strategy allows for control of the microstructure and corresponding lattice distortion by tuning the metal ion composition. Read More

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January 2022

Redox replacement of Ag on MOF-derived Cu/C-nanoparticles on gas diffusion electrodes for electrocatalytic CO2 reduction.

Chemistry 2022 Jan 17. Epub 2022 Jan 17.

Ruhr-Universitat Bochum, Analytische Chemie, Universitätsstr 150, 44780, Bochum, GERMANY.

During the electrochemical CO 2 reduction reaction, bime-tallic tandem catalysts have emerged as a promising strategy to local-ly increase the CO flux for maximizing the conversion rate towards C-C coupled products. Considering this, a novel Cu/C-Ag nanostruc-tured catalyst was prepared by a redox replacement process, where the ratio of both metals can be tuned by the replacement time. An optimum Cu/Ag composition with similarly sized particles showed the highest CO 2 conversion to C 2+ products compared to non-Ag modified gas-diffusion electrodes. Read More

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January 2022

Interfacial compatibility critically controls Ru/TiO metal-support interaction modes in CO hydrogenation.

Nat Commun 2022 Jan 17;13(1):327. Epub 2022 Jan 17.

State Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical Technology, Beijing, 100029, China.

Supports can widely affect or even dominate the catalytic activity, selectivity, and stability of metal nanoparticles through various metal-support interactions (MSIs). However, underlying principles have not been fully understood yet, because MSIs are influenced by the composition, size, and facet of both metals and supports. Using Ru/TiO supported on rutile and anatase as model catalysts, we demonstrate that metal-support interfacial compatibility can critically control MSI modes and catalytic performances in CO hydrogenation. Read More

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January 2022

Discovering the key role of MnO and CeO particles in the FeO catalysts for enhancing the catalytic oxidation of VOC: Synergistic effect of the lattice oxygen species and surface-adsorbed oxygen.

Sci Total Environ 2022 Jan 14:152844. Epub 2022 Jan 14.

Shandong Huanwo Environmental Protection Technology Co., ltd., Binzhou, Shandong 251800, China.

Highly active mesoporous Fe-Mn-Ce catalysts with high specific surface area (S) were synthesized by a modified precipitation process for catalyzing toluene oxidation. The FeMnCe catalyst presents richer surface oxygen species (OS), a higher proportion of Mn and Ce, a higher concentration of lattice defects and oxygen vacancies, the highest O/O ratio, and a superior low-temperature redox property compared with the Fe-Mn binary oxide and FeO and MnO catalysts. The properties contribute to a high catalytic activity to achieve T% of toluene conversion at 264 °C and 185 °C with a gas hourly space velocity (GHSV) at 180,000 and 20,000 mL/(g∙h), respectively. Read More

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January 2022

Selective decomposition of hydrazine over metal free carbonaceous materials.

Phys Chem Chem Phys 2022 Jan 17. Epub 2022 Jan 17.

Dipartimento di Chimica, Università degli Studi di Milano, via Golgi 19, Milano I-20133, Italy.

Herein we report a combined experimental and computational investigation unravelling the hydrazine hydrate decomposition reaction on metal-free catalysts. The study focuses on commercial graphite and two different carbon nanofibers, pyrolytically stripped (CNF-PS) and high heat-treated (CNF-HHT), respectively, treated at 700 and 3000 °C to increase their intrinsic defects. Raman spectroscopy demonstrated a correlation between the initial catalytic activity and the intrinsic defectiveness of carbonaceous materials. Read More

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January 2022

Rational Design of Zinc/Zeolite Catalyst: Selective Formation of p-Xylene from Methanol to Aromatics Reaction.

Angew Chem Int Ed Engl 2022 Jan 17. Epub 2022 Jan 17.

Tsinghua University, Department of Chemical Engineering, CHINA.

The production of p-xylene from methanol to aromatics reaction is challenging. By now, the catalytic stability, which is inversely proportional to the particle size of the zeolite, is always not compatible with p-xylene selectivity, which is inversely proportional to the external acid sites. In this study, based on a nano-sized zeolite, we designed hollow triple-shelled Zn/MFI single crystals using the ultra-dilute liquid-phase growth technique. Read More

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January 2022

Multi-dimensional designer catalysts for negative emissions science (NES): bridging the gap between synthesis, simulations, and analysis.

iScience 2022 Jan 27;25(1):103700. Epub 2021 Dec 27.

Department of Chemistry, University of Utah, Salt Lake City, UT 84112, USA.

Negative emissions technologies will play a critical role in limiting global warming to sustainable levels. Electrocatalytic and/or photocatalytic CO reduction will likely play an important role in this field moving forward, but efficient, selective catalyst materials are needed to enable the widespread adoption of these processes. The rational design of such materials is highly challenging, however, due to the complexity of the reactions involved as well as the large number of structural variables which can influence behavior at heterogeneous interfaces. Read More

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January 2022

Sustained generation of peroxide from the air by carbon nano onion under visible light to combat RNA virus.

J Chem Sci (Bangalore) 2022 12;134(1). Epub 2022 Jan 12.

Department of Applied Chemistry, Ramakrishna Mission Vidyamandira, Belur Math, Howrah, West Bengal 711202 India.

Carbon nano onion (CNO) from dried grass has been synthesized by carbonization in the size range, 20 to 100 nm. This shows catalytic property to transform aerial oxygen under visible light to generate reactive oxygen species (ROS). A concept has been presented herein to show that this CNO even under room light generates hydrogen peroxide which inhibits WSN influenza virus (H1N1). Read More

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January 2022

Catalytic oxidation of VOCs over [email protected] Pd/CoMnO nanosheets supported on hollow AlO microspheres.

J Colloid Interface Sci 2022 Jan 7;613:155-167. Epub 2022 Jan 7.

College of Chemistry, Chemical Engineering and Materials Science, Collaborative Innovation Center of Suzhou Nano Science and Technology, Soochow University, Suzhou 215123, PR China. Electronic address:

Catalytic oxidation is a promising method for removing harmful volatile organic compounds (VOCs). Therefore, exploring high-efficiency catalysts for catalyzing VOCs is of great significance to the realization of an environment-friendly and sustainable society. Here, a series of [email protected] constructed [email protected] microspheres with a hollow hierarchical structure supporting Pd nanoparticles was successfully synthesized. Read More

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January 2022

Ruthenium-nickel-cobalt alloy nanoparticles embedded in hollow carbon microtubes as a bifunctional mosaic catalyst for overall water splitting.

J Colloid Interface Sci 2022 Jan 6;612:710-721. Epub 2022 Jan 6.

Key Laboratory of Superlight Materials and Surface Technology of Ministry of Education, College of Materials Science and Chemical Engineering, Harbin Engineering University, Harbin 150001, PR China. Electronic address:

The development of efficient bifunctional catalysts for both hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) is essential for reducing the cost of hydrogen production by water splitting. Herein, hollow microtubes composed of RuNiCo alloy nanoparticles uniformly embedded in the carbon matrix ([email protected]) are prepared through a simple impregnation followed by reduction. Benefiting from the unique mosaic structure and the synergistic effect between Ru and NiCo, [email protected] achieves more exposed active sites and improved reaction kinetics. Read More

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January 2022

High-efficient carbon dioxide-to-formic acid conversion on bimetallic PbIn alloy catalysts with tuned composition and morphology.

Chemosphere 2022 Jan 12;293:133595. Epub 2022 Jan 12.

Institute for Sustainable Energy, College of Sciences, Shanghai University, Shangda Road 99, Baoshan, Shanghai, 200444, China. Electronic address:

CO electroreduction to value-added chemicals and fuels has gained increasing attention; however, there are only a few catalysts with high performance under mild conditions that can be used in this technique. In this study, single metal Pb, In and bimetallic PbIn catalysts for aqueous CO electroreduction were prepared using a facile 3-step process including PbIn granulation by reducing Pb(NO)/In(NO) aqueous solution with NaBH, calcination in air, and in situ electroreduction. The bimetallic PbIn catalysts had better catalytic performance on CO electroreduction than single metal catalysts. Read More

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January 2022

Hydroboration and reductive amination of ketones and aldehydes with HBpin by a bench stable Pd(II)-catalyst.

Org Biomol Chem 2022 Jan 14. Epub 2022 Jan 14.

Department of Chemistry, Indian Institute of Technology Hyderabad, Kandi, Sangareddy 502284, Telangana, India.

A palladium(II) complex [(κ-{1,2-CH(NCH-CHO)}Pd] (1) supported by a dianionic salen ligand [1,2-CH(NCH-CHO)] (L) was synthesised and used as a molecular pre-catalyst in the hydroboration of aldehydes and ketones. The molecular structure of Pd(II) complex 1 was established by single-crystal X-ray diffraction analysis. Complex 1 was tested as a competent pre-catalyst in the hydroboration of aldehydes and ketones with pinacolborane (HBpin) to produce corresponding boronate esters in excellent yields at ambient temperature under solvent-free conditions. Read More

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January 2022

Copper(II) tetrakis(pentafluorophenyl)porphyrin: highly active copper-based molecular catalysts for electrochemical CO reduction.

Chem Commun (Camb) 2022 Jan 14. Epub 2022 Jan 14.

Division of Applied Chemistry, Graduate School of Engineering Osaka University 2-1 Yamadaoka, Suita, Osaka 565-0871, Japan.

We report a highly active copper-based catalyst for electrochemical CO reduction. Electrochemical analysis revealed that the maximum turnover frequency for CO to CO conversion reached 1 460 000 s at an overpotential () of 0.85 V. Read More

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January 2022

Concentrated Ethanol Electrosynthesis from CO via a Porous Hydrophobic Adlayer.

ACS Appl Mater Interfaces 2022 Jan 14. Epub 2022 Jan 14.

Department of Mechanical and Industrial Engineering, University of Toronto, 5 King's College Road, Toronto, Ontario M5S 3G8, Canada.

Electrochemical CO reduction can convert waste emissions into dense liquid fuels compatible with existing energy infrastructure. High-rate electrocatalytic conversion of CO to ethanol has been achieved in membrane electrode assembly (MEA) electrolyzers; however, ethanol produced at the cathode is transported, via electroosmotic drag and diffusion, to the anode, where it is diluted and may be oxidized. The ethanol concentrations that result on both the cathodic and anodic sides are too low to justify the energetic and financial cost of downstream separation. Read More

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January 2022

Cinchona Alkaloid Derived Iodide Catalyzed Enantioselective Oxidative α-Amination of Carbonyl Compounds toward the Construction of Spiroindolyloxindole.

Org Lett 2022 Jan 13. Epub 2022 Jan 13.

Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, Hubei Engineering Research Center for Biomaterials and Medical Protective Materials, Hubei Key Laboratory of Bioinorganic Chemistry & Materia Medica, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology (HUST), 1037 Luoyu Road, Wuhan 430074, People's Republic of China.

Novel cinchona alkaloid derived iodide catalysts were developed for the enantioselective oxidative α-amination of 2-oxindoles, providing various functionalized spiropyrrolidine oxindoles in high yields and with good enantioselectivities. This iodide/ROOH catalytic system features a one-step synthesis of a catalyst with multiple functionalities, ease of operation, and good scalability, thereby enriching the repertoire of iodide catalysis for enantioselective oxidative coupling reactions. Read More

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January 2022

Chromatic Fulleropyrrolidine as Long-Lived Metal-Free Catalyst for CO2 Photoreduction Reaction.

ChemSusChem 2022 Jan 13. Epub 2022 Jan 13.

National Taiwan University, Center for Condensed Matter Sciences, 1, Sec. 4, Roosevelt Road, 10617, Taipei, TAIWAN.

Conversion of CO 2 into carbonaceous fuels with the aid of solar energy has been an important research subject for decades. Owing to their excellent electron-accepting capacities, fullerene derivatives have been extensively used as n -type semiconductors. This work reports that the fulleropyrrolidine functionalized with 4,7-di(thiophen-2-yl)benzo[c][1,2,5]thiadiazole, abbreviated as DTBT-C 60 , can efficiently catalyze the photoreduction of CO 2 to CO with high selectivity. Read More

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January 2022

Switching Catalyst Selectivity via the Introduction of a Pendant Nitrophenyl Group.

Inorg Chem 2022 Jan 12. Epub 2022 Jan 12.

Department of Chemistry, University of Southern California, Los Angeles, California 90089, United States.

The conversion of abundant small molecules to value-added products serves as an attractive method to store renewable energy in chemical bonds. A family of macrocyclic cobalt aminopyridine complexes was previously reported to reduce CO to CO with 98% faradaic efficiency through the formation of hydrogen-bonding networks and with the number of secondary amines affecting catalyst performance. One of these aminopyridine macrocycles, (NH)(NMe)-bridged calix[4]pyridine (), was modified with a nitrophenyl group to form and metalated with a cobalt(II) precursor to generate , which would allow for probing the positioning and steric effects on catalysis. Read More

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January 2022

-Aminobenzoic acid-capped hematite as an efficient nanocatalyst for solvent-free CO fixation under atmospheric pressure.

Dalton Trans 2022 Jan 12. Epub 2022 Jan 12.

Department of Chemical Sciences, Indian Institute of Science Education and Research (IISER) Kolkata, Mohanpur, West Bengal 741246, India.

Utilization of carbon dioxide by converting it into value-added chemicals is a sustainable remedy approach that stipulates abundant, cheap, non-toxic and efficient catalytic materials. In this study, we have demonstrated the use of -aminobenzoic acid-capped hematite ([email protected]α-FeO) as an efficient nanocatalyst for the conversion of epoxides to cyclic carbonates utilizing CO. The developed [email protected]α-FeO nanocatalyst along with a cocatalyst, tetrabutylammonium iodide (TBAI), was able to convert a variety of epoxide substrates into their corresponding cyclic carbonates under atmospheric pressure and solvent-free conditions. Read More

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January 2022

Strategies for Electrochemically Sustainable H Production in Acid.

Adv Sci (Weinh) 2022 Jan 12:e2104916. Epub 2022 Jan 12.

Fujian Provincial Key Laboratory of Quantum Manipulation and New Energy Materials, College of Physics and Energy, Fujian Normal University, Fuzhou, 350117, China.

Acidified water electrolysis with fast kinetics is widely regarded as a promising option for producing H . The main challenge of this technique is the difficulty in realizing sustainable H production (SHP) because of the poor stability of most electrode catalysts, especially on the anode side, under strongly acidic and highly polarized electrochemical environments, which leads to surface corrosion and performance degradation. Research efforts focused on tuning the atomic/nano structures of catalysts have been made to address this stability issue, with only limited effectiveness because of inevitable catalyst degradation. Read More

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January 2022

Green ammonia synthesis using CeO/RuO nanolayers on vertical graphene catalyst electrochemical route in alkaline electrolyte.

Nanoscale 2022 Jan 12. Epub 2022 Jan 12.

CSIRO Energy, Private Bag 10, Clayton South, Victoria, 3169, Australia.

The electrochemical synthesis of ammonia at ambient temperature and pressure has the potential to replace the conventional process for the production of ammonia. However, the low ammonia yield and poor long-term stability of catalysts for the synthesis of ammonia hinders the application of this technology. Herein, we endeavored to tackle this challenge by synthesizing 3-D vertical graphene (VG) on Ni foam a one-step, low-temperature plasma process, which offered high conductivity and large surface area. Read More

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January 2022

Catalytic production of low-carbon footprint sustainable natural gas.

Nat Commun 2022 Jan 11;13(1):258. Epub 2022 Jan 11.

State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 116023, Dalian, China.

Natural gas is one of the foremost basic energy sources on earth. Although biological process appears as promising valorization routes to transfer biomass to sustainable methane, the recalcitrance of lignocellulosic biomass is the major limitation for the production of mixing gas to meet the natural gas composition of pipeline transportation. Here we develop a catalytic-drive approach to directly transfer solid biomass to bio-natural gas which can be suitable for the current infrastructure. Read More

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January 2022