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High density amorphous ice from cubic ice.

Authors:
Thomas Loerting Ingrid Kohl Werner Schustereder Katrin Winkel Erwin Mayer

Chemphyschem 2006 Jun;7(6):1203-6

Institute of General, Inorganic and Theoretical Chemistry, University of Innsbruck, Austria.

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http://dx.doi.org/10.1002/cphc.200600011DOI Listing
June 2006

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Machine learning models are rapidly becoming widely used to simulate complex physicochemical phenomena with accuracy. Here, we use one such model as well as direct density functional theory (DFT) calculations to investigate the phase equilibrium of water, hexagonal ice (Ih), and cubic ice (Ic), with an eye toward studying ice nucleation. The machine learning model is based on deep neural networks and has been trained on DFT data obtained using the SCAN exchange and correlation functional. Read More

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Institute of Materials Science, TU Bergakademie Freiberg, Gustav-Zeuner-Strasse 5, Freiberg, 09599, Germany.

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Ice in biomolecular cryocrystallography.

Authors:
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Diffraction data acquired from cryocooled protein crystals often include diffraction from ice. Analysis of ice diffraction from crystals of three proteins shows that the ice formed within solvent cavities during rapid cooling is comprised of a stacking-disordered mixture of hexagonal and cubic planes, with the cubic plane fraction increasing with increasing cryoprotectant concentration and increasing cooling rate. Building on the work of Thorn and coworkers [Thorn et al. Read More

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Routes to cubic ice through heterogeneous nucleation.

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Proc Natl Acad Sci U S A 2021 Mar;118(13)

Department of Chemistry, University of Cambridge, Cambridge CB2 1EW, United Kingdom

The freezing of water into ice is one of the most important processes in the physical sciences. However, it is still not understood at the molecular level. In particular, the crystallization of cubic ice ([Formula: see text])-rather than the traditional hexagonal polytype ([Formula: see text])-has become an increasingly debated topic. Read More

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Water has a rich phase diagram with several crystals, as confirmed by experiments. High-pressure and high-temperature water is of interest for Earth's mantle and exoplanetary investigations. It is in this region of the phase diagram of water that new plastic crystal phases of water have been revealed via computer simulations by both classical forcefields and ab initio calculations. Read More

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